Here's something to get you started:
var dspStartsWithR = From row in myDataTable.Rows
Where (string)row("DSP Name").StartsWith("R|")
var dspStartsWithS = From row in myDataTable.Rows
Where (string)row("DSP Name").StartsWith("S|")
Once you get your results you're going to have to do some combination of Substring to strip out the characters you don't need, do comparisons, etc. My C# is rusty so sorry if the code isn't quite right.