The problem is fixed:
conn = new SqlConnection(ConfigurationManager.ConnectionStrings["OPSConnection"].ConnectionString);
string query = "SELECT SUM(Pick.Colli) AS TotalPick, SUM(Pack.Colli) AS TotalPack, Pack.Person_pack AS persoon FROM Pick CROSS JOIN Pack WHERE person_pack = 'annem2' GROUP BY person_pack";
SqlCommand cmd = new SqlCommand(query, conn);
conn.Open();
SqlDataReader sqlReader = cmd.ExecuteReader();
Series Series1 = new Series();
Chart1.Series.Add(Series1);
Series1.YValuesPerPoint = 2;
DataTable dt = new DataTable();
dt.Columns.Add(new DataColumn("Personen"));
dt.Columns.Add(new DataColumn("Total"));
while (sqlReader.Read())
{
dt.Rows.Add(sqlReader.GetValue(2),sqlReader.GetValue(0));
dt.Rows.Add(sqlReader.GetValue(2), sqlReader.GetValue(1));
}
Chart1.Series[0].XValueMember = "Personen";
Chart1.Series[0].YValueMembers = "Total";
Chart1.DataSource = dt;
Chart1.Series[0].ChartType = SeriesChartType.Pie;
Chart1.Series[0].ToolTip = "#VALY";
Chart1.DataBind();
conn.Close();