According to this article by Microsoft, Only members of the sysadmin fixed server role can create and alter UNSAFE assemblies.
You will need to add your current login to the sysadmin fixed server role.
I don't have my management studio available at this time, but I believe this will work:
USE YOURDATABASENAME
GO
EXEC sp_addsrvrolemember 'YOURUSERNAME', 'sysadmin';