You have a repeated set of controls. Therefore you need a corresponding repeated set of variables that store these values. I suggest creating a class where you can store a variable (or property) set.
Public Class ControlSet
Public Property Description As String
Public Property Type As String
Public Property XFieldName As String
Public Property Colour As String
End Class
Create an array that holds these values
Dim Values = New ControlSet(ddlFieldNames.SelectedIndex) {}
And retrieve the values in a loop
For i As Integer = 0 To Values.Length - 1
Values(i).Description = CType(divDesc.FindControl("txt-" & Convert.ToString(i + 1)), TextBox).Text
Values(i).Type = CType(divChart.FindControl("comboChart-" & Convert.ToString(i + 1)), RadComboBox).SelectedValue
Values(i).XFieldName = ...
...
Next
Also use the ID of the control; this helps to avoid confusion in case you have several controls of the same type.