You'd want to check the time whether it's before or after 12:00 noon. If it's 11:59:59 or less, add it to the previous day. Anything after, current day. Create a formula using something like this
IF TIME({yourdatetime}) <= TIME(11,59,59) THEN
DATE({yourdatetime}) - 1
ELSE
DATE({yourdatetime})
Then group by the formula and format the group header for just the date.