This DID FIX the problem. I'm still limited to 2 GB of memory from within VS 2013 in debug mode. However, when deploying to IIS7.5, 2008 R2 Server, and App. Pool of dot net 4.0x, I can use a lot more memory for my website. It took the following setting in my web.config. I now need to bump my physical from 8 to 16 GBs; But, that is a different story. Solution:
<gcAllowVeryLargeObjects enabled="true" />
https://msdn.microsoft.com/en-us/library/hh285054(v=vs.110).aspx