if you are using aforge libraries, you can utilize his extension too, named Accord.Net.
Accord.Net is similar at Aforge, you install it, add the references at your project and you are done.
After that you can use the simply the RawMoments by passing the target image, and after you can use them to compute CentralMoments
At this point you can get the angle of your image with the method of CentralMoments GetOrientation() and you get the angle.
I used it on an hand-gestures recognition project and worked like a charm.
UPDATE: I have just checked that GetOrientation get only the angle but not the direction. So an upside-down image have the same angle of the original. A fix, can be the pixel counting, but this time you will get only 2 (worst case) samples to check and not 360 (worst case) samples.
Update2
If you have a lot of samples, i suggest you to filter them with the size of the rotated image. Example: I get the image, i see that is in a Horizontal position (90°) i rotate it of 90° and now i have the original width and heigth that i can utilize to skip the samples that are not similar, like:
If (Founded.Width != Sample.Width) //You can add a range too if in case during
Continue; //the rotation are added some pixels